Journal of Nuclear Physics, Material Sciences, Radiation and Applications
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Hydrochemistry and Uranium Concentration in Brackish Groundwater from an Arid Zone, Chihuahua, Mexico
In arid zones, the principal water supply is from groundwater, which can present high concentration of salts, heavy metals, and radioactive elements. The aim of the study was to determine isotopic uranium concentration in groundwater samples with high concentration of salts and its association with other chemical species. Samples were taken from wells with high salt content. The 238,234U radioisotope concentrations were determined by liquid scintillation and alpha-particle spectrometry. In addition, the physical-chemical parameters were recorded in situ; whereas the dissolved ions and elemental composition were measured by UV-Vis and X-ray fluorescence spectrophotometry, respectively. To obtain isotopic uranium concentrations, three radiochemistry procedures were carried out. An ANOVA test was performed to compare the results from procedures, as well as an analysis of Pearson correlation was used between parameters to obtain their associations. Statistically, the U isotopic concentrations did not show differences (p-value 0.82) between procedures. 238U and 234U showed mean concentrations of 6.7 mBq mL-1 and 16.6 mBq mL-1, respectively, with an Activity Ratioby up 7.2. The groundwater under study showed high concentration of TDS, calcium, sulphate, chloride, nitrate, and nitrite. Isotopic U concentrations tend to increase with NO3>Zn>Cl>Br>SO4>Cu>T>SDT>P; meanwhile their contents decrease with T>Cl->NO2>Fe. These findings help us to understand the uranium behavior in groundwater with high salt contents as well as the influence of agricultural supplies on chemical species presents in groundwater
Optimization of the Position of the CR-39 Polycarbonate Sheet Inside the Solid State Track Detector “Measuring Device” Through Computational Fluid Dynamics Technique
The “measuring device” is one of the most reliable, efficient and economic indoor radon dosimeters that exist. This device was developed by the Proyecto de Aplicaciones de la Dosimetría (PAD) at the Physics Institute of UNAM (IF-UNAM) and consists of a transparent rigid plastic cup, a CR-39 polycarbonate sheet and a standard size metal clip that is used to hold the polycarbonate in the center of the cup. The cup is wrapped and covered with a low-density polyurethane protector in order to prevent the detector from being irradiated by ionizing particles found in the environment. In this work, an analysis was carried out that allowed to understand how the radon concentration on the polycarbonate sheet varies when its height is changed with respect to the base of the plastic cup, in order to understand what position increase the probability of interaction between radon and the surface of the detector. For the development of this work, four computational simulations were performed with the technique called Computational Fluid Dynamics (CFD). The results shows that as the CR-39 is positioned more closed to the base of the cup, the probability of interaction of the radon and the detector increase. Based on these results it is concluded that, when there is a limit in the time in which a measuring device can be placed in the zone where it is desired to quantify indoor radon, it is recommended to collocated the CR-39 at 1 cm with respect to the base of the cup
Radon Dose Determination and Radiological Risk in Some Mexican Caves with CR-39 Detectors
Radon (222Rn) is a radioactive gas, from the 238U decay chain, that contributes in large part of the natural radiation dose to which humans are exposed. Radon is the second cause of lung cancer after tobacco. The US-EPA considers a concentration of 148 Bq/m3 for homes and 400 Bq/m3 for workplaces as the reference level. Caves are closed spaces where 222Rn, which emanates from the surrounding minerals and rocks, can accumulate and reaches large concentrations that can represent a health risk for the guides, speleologists and visitors who spend time in these spaces. This work uses the previously recorded radon concentrations in 8 caves in Mexico and calculates the average dose range and the average annual dose for each of them with the “Wise” public domain program (http://www.wise-uranium.org/rdcrn.html) to determine the level of radiological risk with 2,000 1,000 and 500 working hours per year. Karmidas cave had the highest average 222Rn concentration with 27,633.3 Bq/m3 and for 2,000 working hours per year an average annual dose rate of 347.1 mSv/y. Los Riscos cave had the lowest average concentration with 384.7 Bq/m3 and for 2,000 working hours per year an average annual dose rate of 4.832 mSv/y. These results show that all the caves studied present values,with 2,000 working hours per year, that exceed 3 mSv/y for workplaces and must be considered by the people who work in these places. A casual tourist visiting the caves does not present any radiological risk, while guides and speleologists should consider it
Appearance / Disappearance of Magic Number in Light Nuclei
The shell structure of a nucleus is important to study their observed characteristic features. The classic magic numbers are successful in explaining the nuclear properties for nuclei lying near the stability line. The advent of radioactive ion beam facilities has permitted to examine nuclei in their extreme proton to neutron ratio. The light exotic nuclei were found to exhibit unique shell closure behaviour which is different from the medium mass nuclei near the stability line. The two nucleon separation energy difference systematics was used as a probe to study the magic character of light nuclei. New proton and neutron magic numbers were predicted among the available even Z isotopes and even N isotones. For certain systems, the classic magic numbers were found to be non-magic, while for some systems the magic property is retained even at the drip lines. The shell closure behaviour predicted is found to depend on the version of the mass table
PADC-NTM Applied in 7Li+Pb at 31 MeV Reaction Products Study
Passive nuclear track methodology (NTM) is applied to study charged particles products of the reaction 7Li+Pb at ~ 31 MeV. It is a contribution to the 8pLP Project (LNL-INFN-Italy) in where we show an alternative approach to register charged particle from reaction fragments by PADC detection. The main advantage is that the passive system integrates data over the whole experiment and has its importance for low rate reaction processes. Reaction products as well as scattered beam particles are determined from track shape analysis. Some limitations are inherent to NTM since a priori knowledge is required to correlate track size distribution given by each type of particle emerging from the target. Results show that the passive technique gives useful information when applied in reaction data interpretation for a relatively large range of particle types
Effect of Laser Radiation on Biomolecules
Time of flight laser photoionization has been used to study the response of some molecules of biological interest under laser radiation. One of the questions of great interest today is the effect of radiation on DNA and RNA molecules. Damage to these molecules can be caused directly by radiation or indirectly by secondary electrons created by radiation. As response of the radiation field fragmentation process can occur producing different ions with kinetic energies of a few electron volts. In this paper we present the results of the interaction of 355nm laser with the nitrogen bases adenine(A) and uracil(U) using time-of-flight spectrometry and the comparison of experimental results on the effects of laser radiation in (A) and (U) belonging to two different ring groups, purines and pyrimidines respectively, which are linked to form the AU pair of the RNA
Preliminary Measurements of Be-10/Be-7 Ratio in Rainwater for Atmospheric Transport Analysis
The meteoric cosmogenic beryllium has been used as an essential geophysical tracer in the analysis of atmospheric flows and erosion soils since 1960. The first measurements Be-7 and Be-10 concentrations in rainwater from Mexico, have been carried out by using gamma decay spectroscopy and AMS techniques, respectively for each isotope. With this it was possible to report a preliminar value for the Be-10/Be-7 isotopic ratio in such environmental samples. The present work described preliminary results related to rainwater collected at mountain and metropolitan areas. Results are compared with predictions and previous measurements for both radioisotopes, observing a very sensible behavior particularly for the case of Be-7 activities
Cluster radioactivity in superheavy nuclei 299-306122
Cluster radioactivity is an intermediate between alpha decay and spontaneous fission. It is also an exotic decay obtained in superheavy nuclei. When a cluster decay is detected in superheavy nuclei, the daughter nuclei is having near or equal to doubly magic nuclei. We have investigated cluster decay of isotopes of He, Li, Be, Ne, N, Mg, Si, P, S, Cl, Ar and Ca in the superhaevy nuclei region 299-306122. We have also compared the logarithmic half-lives of cluster decay with that of other models such as Univ [1], NRDX [2], UDL [3] and Horoi [4]. From this study it is concluded that cluster decay of 4He, 22Ne, 26Mg, 28Si 30Si, 34S, 40Ca and 46Ca are having shorter logarithmic half-lives compared to exotic cluster decay modes
On the role of nuclear quantum gravity in understanding nuclear stability range of Z = 2 to 118
To understand the mystery of final unification, in our earlier publications, we proposed two bold concepts: 1) There exist three atomic gravitational constants associated with electroweak, strong and electromagnetic interactions. 2) There exists a strong elementary charge in such a way that its squared ratio with normal elementary charge is close to reciprocal of the strong coupling constant. In this paper we propose that, ℏc can be considered as a compound physical constant associated with proton mass, electron mass and the three atomic gravitational constants. With these ideas, an attempt is made to understand nuclear stability and binding energy. In this new approach, with reference to our earlier introduced coefficients k = 0.00642 and f = 0.00189, nuclear binding energy can be fitted with four simple terms having one unique energy coefficient. The two coefficients can be addressed with powers of the strong coupling constant. Classifying nucleons as ‘free nucleons’ and ‘active nucleons’, nuclear binding energy and stability can be understood. Starting from , number of isotopes seems to increase from 2 to 16 at and then decreases to 1 at For Z >= 84, lower stability seems to be, Alower=(2.5 to 2.531)Z
Structural Variations Induced by Temperature Changes in Rotavirus VP6 Protein Immersed in an Electric Field and Their Effects on Epitopes of The Region 300-396
Rotavirus diarrhea is an infectious intestinal disease that causes about 215 thousand deaths annually in infants under five years old. This virus is formed by three layers of concentric proteins that envelop its genome, from which VP6 structural protein is the most conserved among rotavirus serotypes and an excellent vaccine candidate. Recent studies have shown that structural proteins are susceptible to losing their biological function when their conformation is modified by moderate temperature increments, and in the case of VP6, its antigen efficiency decreases. We performed an in silicoanalysis to identify the structural variations in the epitopes 301-315, 357-366, and 376-384 of the rotavirus VP6 protein -in a hydrated medium- when the temperature is increased from 310 K to 322 K. In the latter state, we applied an electric field equivalent to a low energy laser pulse and calculated the fluctuations per amino acid residue. We identified that the region 301-315 has greater flexibility and density of negative electrical charge; nevertheless, at 322 K it experiences a sudden change of secondary structure that could decrease its efficiency as an antigenic determinant. The applied electric field induces electrical neutrality in the region 357-366, whereas in 376-384 inverts the charge, implying that temperature changes in the range 310 K-322 K are a factor that promotes thermoelectric effects in the VP6 protein epitopes in the region 300-396