1,720,964 research outputs found

    Ga particle templated assembly dataset

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    SEM image set for: Waters, Robin et al (2016) Templated assembly of metal nanoparticle films on polymer substrates. Applied Physics Letters.</span

    Gallium phase change as a mechanism for resonance tuning in photonic nanostructures

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    This thesis covers contributions to the field of electromagnetic metamaterials, a broad, dynamic area that has produced a considerable array of new phenomena and is now looking to the prospect of tuning and switching the characteristics of novel materials and surfaces, using many means including thermal and electromagnetic excitation, in order to extend their usefulness and to enable their application in practical devices. In particular, this work develops materials that allow electromagnetic and thermal control of material optical properties and methods that facilitate the use of metasurface physics on macroscopic scales.The reversible photoconductivity effect produced by phase coexistence in an elemental metal has been enhanced in a metamaterial for the first time. A gap plasmon absorber type metasurface was developed to enhance the photoconductivity of a gallium metal interface under near infrared illumination, achieving an order of magnitude increase in the strength of the phenomenon in a pump-probe experiment. The enhanced nonlinearity displayed at the pump wavelength of 1310nm corresponds to an effective nonlinear dielectric susceptibility x(3) of greater than 1 × 10−8 m3 V−2.Competing descriptions of the mechanism behind the reversible photoconductivity effect in elemental gallium, including an analytic model based on heat transfer, a non-thermal model of light-induced excitation, full finite element simulation and a novel cellular automaton method have been implemented and compared. These models have been adapted and applied to the metasurface-enhanced interface for the enhancement of the effect. It was found that an exclusively thermodynamic theoretical treatment of laser heating is insufficient to explain the magnitude of the observed excitation and hence an additional possibly non-thermal photoexcited mechanism must contribute.Processing methods were developed for the testing of nano-imprint metamaterial manufacturing with liquid metals under controlled environmental conditions, using a custom-built pressure controlled processing chamber. Using this methodology a feasibility study of the production of a nanoimprinted liquid metal photonic structure was conducted, successfully demonstrating the infiltration of nanoscale gratings of period 600nm with liquid gallium and optical switching of the resulting composite interface.The templated deposition of ordered arrays of gallium nanoparticles on structured substrates has been demonstrated for the first time. Bulk gallium was thermally evaporated onto substrates structured with gratings and checkerboard-type patterns of period 200 to 1600nm. Fourier and image analysis of the produced ordering shows a pronounced tendency for the nanoparticle growth to align with the substrate patterns in both positional frequency and diameter. Such ordered arrays of metallic particles could form an active medium as a component of a plasmonic metamaterial

    Adaptive photonic meta-surfaces exploiting interfacial phase change in elemental gallium

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    Surface-driven metallization in a nanoscale layer of elemental gallium forming the backplane of a photonic metamaterial absorber provides a mechanism for reversible all-optical and thermo-optical tuning of resonant response

    Optically switchable gallium metasurfaces

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    We report on the first experimental demonstration of an optically nonlinear gallium-based photonic metamaterial, in which a reversible light-induced transition between solid and liquid phases occurring in a confined nanoscale surface layer of the metal drives significant changes in reflectivity, offering high contrast all-optical switching in the visible/near-infrared range at low, µW/µm2, optical excitation intensities

    All-optical switching of photonic metamaterials enabled by surface-mediated phase transitions in gallium

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    Reversible, optically-induced surface metallization in a nanoscale layer of elemental gallium forming the backplane of a photonic metamaterial absorber provides a mechanism for a strong, resonantly enhanced reflective optical nonlinearity at µW/µm2 intensities

    Going Beyond Counting First Authors in Author Co-citation Analysis

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    The present study examines one of the fundamental aspects of author co-citation analysis (ACA) - the way co-citation counts are defined. Co-citation counting provides the data on which all subsequent statistical analyses and mappings are based, and we compare ACA results based on two different types of co-citation counting - the traditional type that only counts the first one among a cited work's authors on the one hand and a non-traditional type that takes into account the first 5 authors of a cited work on the other hand. Results indicate that the picture produced through this non-traditional author co-citation counting contains more coherent author groups and is therefore considerably clearer. However, this picture represents fewer specialties in the research field being studied than that produced through the traditional first-author co-citation counting when the same number of top-ranked authors is selected and analyzed. Reasons for these effects are discussed

    Variations on the Author

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    “Variations on the Author” discusses two of Eduardo Coutinho’s recent films (Um Dia na Vida, from 2010, and Últimas Conversas, posthumously released in 2015) and their contribution to the general question of documentary authorship. The director’s filmography is characterized by a consistent yet self-effacing form of authorial self-inscription: Coutinho often features as an interviewer that rather than express opinions propels discourses; an interviewer that is good at listening. This mode of self-inscription characterizes him as an author who is not expressive but who is nonetheless markedly present on the screen. In Um Dia na Vida, however, Coutinho is completely absent form the image, while Últimas Conversas, on the contrary, includes a confessional prologue that moves the director from the margins to the center of his films. This article examines the ways in which these works stand out in the filmography of a director who offers new insights into the notion of cinematic authorship

    Appropriate Similarity Measures for Author Cocitation Analysis

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    We provide a number of new insights into the methodological discussion about author cocitation analysis. We first argue that the use of the Pearson correlation for measuring the similarity between authors’ cocitation profiles is not very satisfactory. We then discuss what kind of similarity measures may be used as an alternative to the Pearson correlation. We consider three similarity measures in particular. One is the well-known cosine. The other two similarity measures have not been used before in the bibliometric literature. Finally, we show by means of an example that our findings have a high practical relevance.information science;Pearson correlation;cosine;similarity measure;author cocitation analysis
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