1,720,975 research outputs found
Bimodal Functionality of Highly Conductive Nanostructured Silver Film Towards Improved Performance of Photosystem I-Based Graphene Photocathode
Unlu, Cumhur Gokhan/0000-0003-2554-5886; Szalkowski, Marcin/0000-0002-7514-5875; Kowalska, Dorota/0000-0002-9994-1075; Ocakoglu, Kasim/0000-0003-2807-0425; Harputlu, Ersan/0000-0002-2140-9070; Izzo, Miriam/0000-0003-4586-610XWe present the novel design of photosystem I (PSI)-based biosolar cell, whereby conductive transparent electrode materials, such as ITO or FTO, are replaced with glass covered with silver island film. This nanostructured metallic layer combines high electric conductance with enhancing the absorption efficiency of the PSI biocatalyst via the plasmonic effect. We demonstrate strong enhancement of the photocurrent generated in the biohybrid electrode composed of oriented layers of PSI reaction centers due to plasmonic interactions of the PSI fluorophores and redox centres with the conductive silver island film.Polish National Center for Research and Development [DZP/POLTUR-1/50/2016, 5/POLTUR-1/2016]; Scientific and Technological Research Council of Turkiye, TUBITAK [215M389, 123N061/SUNCOCAT]; Poland's National Science Centre, Solar driven chemistry 2 grant (SUNCOCAT) [2022/04/Y/ST4/00107]JK, MK, MI, MS, DK and SM acknowledge the financial support for this work from the Polish National Center for Research and Development (grant no. DZP/POLTUR-1/50/2016, agreement no. 5/POLTUR-1/2016 to JK and SM), while KO, CGU and EH are supported by the Scientific and Technological Research Council of Turkiye, TUBITAK (grant no. 215M389 and 123N061/SUNCOCAT to KO) within the framework of 1st Bilateral Polish-Turkish POLTUR program. Some of this work was supported by Poland's National Science Centre, Solar driven chemistry 2 grant (SUNCOCAT grant no. 2022/04/Y/ST4/00107 to JK)
Predicting the impact of temperature dependent multi-phonon relaxation processes on the photon avalanche behavior in Tm3+: NaYF4 nanoparticles
Photon avalanche (PA) is an anti-Stokes process in which lanthanide-doped materials can emit upconverted luminescence in a highly non-linear manner. PA was recently demonstrated in thulium (III)-doped NaYF4 colloidal nanoparticles at room temperature, with reported nonlinearities (power factors) exceeding 30. Importantly, good rate-equations model agreement with experimental data was achieved, which enabled the derivation of the rates of energy transfer processes, providing a foundation for further developments and optimization of similar materials and their new applications. In order to apply PA to, for example, luminescent (nano)thermometry, we need to have a better understanding of the susceptibility of photon avalanche phenomenon to temperature variation. For this purpose, we study how the temperature and energy-gap-dependent multiphonon relaxation and inter-ionic energy transfer processes affect the photon avalanche behavior. As a result of these simulations, high susceptibility to temperature changes with relative sensitivity over 40 %⋅K−1 above 400 K (up to 15 %⋅K−1at room temperature) was noted. Moreover, by knocking-out the temperature dependences of the individual processes involved in the PA, we found the temperature dependence of the multiphonon relaxation of the intermediate F34 state to the ground state to be the primary one responsible for the simulated temperature dependence of PA emission. This process is observed to be more significant than temperature dependencies of energy looping and phonon assisted ground state non-resonant absorption. Although there are challenges with a single band technique, these results still show the great potential, especially when used ratiometrically with different excitation wavelengths.
Going Beyond Counting First Authors in Author Co-citation Analysis
The present study examines one of the fundamental aspects of author co-citation analysis (ACA) - the way co-citation
counts are defined. Co-citation counting provides the data on which all subsequent statistical analyses and mappings
are based, and we compare ACA results based on two different types of co-citation counting - the traditional type that
only counts the first one among a cited work's authors on the one hand and a non-traditional type that takes into
account the first 5 authors of a cited work on the other hand. Results indicate that the picture produced through this non-traditional author co-citation counting contains more coherent author groups and is therefore considerably clearer. However, this picture represents fewer specialties in the research field being studied than that produced through the traditional first-author co-citation counting when the same number of top-ranked authors is selected and analyzed. Reasons for these effects are discussed
Variations on the Author
“Variations on the Author” discusses two of Eduardo Coutinho’s recent films (Um Dia na Vida, from 2010, and Últimas Conversas, posthumously released in 2015) and their contribution to the general question of documentary authorship. The director’s filmography is characterized by a consistent yet self-effacing form of authorial self-inscription: Coutinho often features as an interviewer that rather than express opinions propels discourses; an interviewer that is good at listening. This mode of self-inscription characterizes him as an author who is not expressive but who is nonetheless markedly present on the screen. In Um Dia na Vida, however, Coutinho is completely absent form the image, while Últimas Conversas, on the contrary, includes a confessional prologue that moves the director from the margins to the center of his films. This article examines the ways in which these works stand out in the filmography of a director who offers new insights into the notion of cinematic authorship
Appropriate Similarity Measures for Author Cocitation Analysis
We provide a number of new insights into the methodological discussion about author cocitation analysis. We first argue that the use of the Pearson correlation for measuring the similarity between authors’ cocitation profiles is not very satisfactory. We then discuss what kind of similarity measures may be used as an alternative to the Pearson correlation. We consider three similarity measures in particular. One is the well-known cosine. The other two similarity measures have not been used before in the bibliometric literature. Finally, we show by means of an example that our findings have a high practical relevance.information science;Pearson correlation;cosine;similarity measure;author cocitation analysis
Dispelling the Myths Behind First-author Citation Counts
We conducted a full-scale evaluative citation analysis study of scholars in the XML research field to explore just how different from each other author rankings resulting from different citation counting methods actually are, and to demonstrate the capability of emerging data and tools on the Web in supporting more realistic citation counting methods. Our results contest some common arguments for the continued
use of first-author citation counts in the evaluation of scholars, such as high correlations between author rankings by first-author citation counts and other citation
counting methods, and high costs of using more realistic citation counting methods that are not well-supported by the ISI databases. It is argued that increasingly available digital full text research papers make it possible for citation analysis studies to go beyond what the ISI databases have directly supported and to employ more
sophisticated methods
koamabayili/VECTRON-author-checklist: VECTRON author checklist
We have done our best to complete the author checklist relating to the use of animals in the hut study. Note that the objective for the hut study was to evaluate the IRS treatment applications for residual efficacy against Anopheles mosquitoes, including the local An. coluzzii mosquito population. Cows were only used to attract mosquitoes into the huts and no tests were carried out directly on the cows. The author checklist is intended for use with studies where experiments are carried out on animals, which is why we have had such difficulty in completing this for the hut study, as many of the questions do not relate to how the cows were used
Author-wise bibliometric analysis based on entropy.
Author-wise bibliometric analysis based on entropy.</p
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