1,721,026 research outputs found

    Anion exchange in inorganic perovskite nanocrystal polymer composites

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    We demonstrate a facile, low-cost and room-temperature method of anion exchange in cesium lead bromide nanocrystals (CsPbBr3 NCs), embedded into a polymer matrix. The anion exchange occurs upon exposure of the solid CsPbBr3 NCs/PDMS nanocomposite in controlled anion precursor gas atmosphere. The rate and extent of the anion exchange reaction can be controlled via the variation of either the exposure time or the relative concentration of the anion precursor gas. Post-synthesis chemical transformation of perovskite nanocrystal-polymer composites is not readily achievable using conventional methods of anion exchange, which renders the gas-assisted strategy extremely useful. We envisage that this work will enable the development of solid-state perovskite NCs optoelectronic devices

    Going Beyond Counting First Authors in Author Co-citation Analysis

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    The present study examines one of the fundamental aspects of author co-citation analysis (ACA) - the way co-citation counts are defined. Co-citation counting provides the data on which all subsequent statistical analyses and mappings are based, and we compare ACA results based on two different types of co-citation counting - the traditional type that only counts the first one among a cited work's authors on the one hand and a non-traditional type that takes into account the first 5 authors of a cited work on the other hand. Results indicate that the picture produced through this non-traditional author co-citation counting contains more coherent author groups and is therefore considerably clearer. However, this picture represents fewer specialties in the research field being studied than that produced through the traditional first-author co-citation counting when the same number of top-ranked authors is selected and analyzed. Reasons for these effects are discussed

    Variations on the Author

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    “Variations on the Author” discusses two of Eduardo Coutinho’s recent films (Um Dia na Vida, from 2010, and Últimas Conversas, posthumously released in 2015) and their contribution to the general question of documentary authorship. The director’s filmography is characterized by a consistent yet self-effacing form of authorial self-inscription: Coutinho often features as an interviewer that rather than express opinions propels discourses; an interviewer that is good at listening. This mode of self-inscription characterizes him as an author who is not expressive but who is nonetheless markedly present on the screen. In Um Dia na Vida, however, Coutinho is completely absent form the image, while Últimas Conversas, on the contrary, includes a confessional prologue that moves the director from the margins to the center of his films. This article examines the ways in which these works stand out in the filmography of a director who offers new insights into the notion of cinematic authorship

    Appropriate Similarity Measures for Author Cocitation Analysis

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    We provide a number of new insights into the methodological discussion about author cocitation analysis. We first argue that the use of the Pearson correlation for measuring the similarity between authors’ cocitation profiles is not very satisfactory. We then discuss what kind of similarity measures may be used as an alternative to the Pearson correlation. We consider three similarity measures in particular. One is the well-known cosine. The other two similarity measures have not been used before in the bibliometric literature. Finally, we show by means of an example that our findings have a high practical relevance.information science;Pearson correlation;cosine;similarity measure;author cocitation analysis

    Dispelling the Myths Behind First-author Citation Counts

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    We conducted a full-scale evaluative citation analysis study of scholars in the XML research field to explore just how different from each other author rankings resulting from different citation counting methods actually are, and to demonstrate the capability of emerging data and tools on the Web in supporting more realistic citation counting methods. Our results contest some common arguments for the continued use of first-author citation counts in the evaluation of scholars, such as high correlations between author rankings by first-author citation counts and other citation counting methods, and high costs of using more realistic citation counting methods that are not well-supported by the ISI databases. It is argued that increasingly available digital full text research papers make it possible for citation analysis studies to go beyond what the ISI databases have directly supported and to employ more sophisticated methods

    Author Index

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    Programming the assembly of gold nanoparticles on graphene oxide sheets using DNA

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    We present a new method to program the covalent binding of gold nanoparticles onto graphene oxide sheets. The binding selectivity is driven by the synergy of chemically modified oligonucleotides, grafted onto the surfaces of nanoparticles and graphene oxide. In the presence of a templating complementary DNA strand, nanoparticles are brought near the surface of the graphene oxide. Once in close proximity, the DNA strands are ligated to create a permanent link between the nanoparticles and graphene oxide, ensuring stability of the system even during DNA melting conditions. Due to the selectivity and specificity of DNA, a second layer of gold nanoparticles of different size can be grafted on the top of the first layer of particles. The simplicity of this new method allows for its universal applicability when the formation of highly programmable, covalently linked hybrid nanoparticle–graphene oxide structures is a necessit

    koamabayili/VECTRON-author-checklist: VECTRON author checklist

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    We have done our best to complete the author checklist relating to the use of animals in the hut study. Note that the objective for the hut study was to evaluate the IRS treatment applications for residual efficacy against Anopheles mosquitoes, including the local An. coluzzii mosquito population. Cows were only used to attract mosquitoes into the huts and no tests were carried out directly on the cows. The author checklist is intended for use with studies where experiments are carried out on animals, which is why we have had such difficulty in completing this for the hut study, as many of the questions do not relate to how the cows were used

    Plasmonic backscattering effect in high-efficient organic photovoltaic devices

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    A universal strategy for efficient light trapping through the incorporation of gold nanorods on the electron transport layer (rear) of organic photovoltaic devices is demonstrated. Utilizing the photons that are transmitted through the active layer of a bulk heterojunction photovoltaic device and would otherwise be lost, a significant enhancement in power conversion efficiency (PCE) of poly[N-9?-heptadecanyl-2,7-carbazole-alt-5,5-(4?,7?-di-2-thienyl-2?,1?,3?-benzothiadiazole)]:phenyl-C71-butyric acid methyl ester (PCDTBT:PC71BM) and poly[[4,8-bis[(2-ethylhexyl)oxy]benzo[1,2-b:4,5-b?]dithiophene-2,6-diyl][3-fluoro-2-[(2-ethylhexyl)carbonyl]thieno[3,4-b] thiophenediyl]] (PTB7):PC71BM by ?13% and ?8%, respectively. PCEs over 8% are reported for devices based on the PTB7:PC71BM blend. A comprehensive optical and electrical characterization of our devices to clarify the influence of gold nanorods on exciton generation, dissociation, charge recombination, and transport inside the thin film devices is performed. By correlating the experimental data with detailed numerical simulations, the near-field and far-field scattering effects are separated of gold nanorods (Au NRs), and confidently attribute part of the performance enhancement to the enhanced absorption caused by backscattering. While, a secondary contribution from the Au NRs that partially protrude inside the active layer and exhibit strong near-fields due to localized surface plasmon resonance effects is also observed but is minor in magnitude. Furthermore, another important contribution to the enhanced performance is electrical in nature and comes from the increased charge collection probability
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