1,720,981 research outputs found
Boiling a Unitary Fermi Liquid
We study the thermal evolution of a highly spin-imbalanced, homogeneous Fermi gas with unitarity limited interactions, from a Fermi liquid of polarons at low temperatures to a classical Boltzmann gas at high temperatures. Radio-frequency spectroscopy gives access to the energy, lifetime, and short-range correlations of Fermi polarons at low temperatures T. In this regime, we observe a characteristic T^{2} dependence of the spectral width, corresponding to the quasiparticle decay rate expected for a Fermi liquid. At high T, the spectral width decreases again towards the scattering rate of the classical, unitary Boltzmann gas, ∝T^{-1/2}. In the transition region between the quantum degenerate and classical regime, the spectral width attains its maximum, on the scale of the Fermi energy, indicating the breakdown of a quasiparticle description. Density measurements in a harmonic trap directly reveal the majority dressing cloud surrounding the minority spins and yield the compressibility along with the effective mass of Fermi polarons.United States. National Science Foundation. (Award PHY-1734011)United States. National Science Foundation. (Award PHY-1506019)United States. Air Force. Office of Scientific Research (Grant FA9550-16-1-0324)United States. Air Force. Office of Scientific Research. Multidisciplinary University Research Initiative (Grant FA9550-14-1-0035)United States. Office of Naval Research (Grant N00014-17-1-2257
Cascade of Solitonic Excitations in a Superfluid Fermi gas: From Planar Solitons to Vortex Rings and Lines
We follow the time evolution of a superfluid Fermi gas of resonantly interacting [superscript 6]Li atoms after a phase imprint. Via tomographic imaging, we observe the formation of a planar dark soliton, its subsequent snaking, and its decay into a vortex ring, which, in turn, breaks to finally leave behind a single solitonic vortex. In intermediate stages, we find evidence for an exotic structure resembling the Φ soliton, a combination of a vortex ring and a vortex line. Direct imaging of the nodal surface reveals its undulation dynamics and its decay via the puncture of the initial soliton plane. The observed evolution of the nodal surface represents dynamics beyond superfluid hydrodynamics, calling for a microscopic description of unitary fermionic superfluids out of equilibrium.National Science Foundation (U.S.)United States. Army Research Office. Multidisciplinary University Research Initiative on AtomtronicsUnited States. Air Force Office of Scientific Research. Presidential Early Career Award for Scientists and EngineersUnited States. Air Force Office of Scientific Research. Multidisciplinary University Research Initiative on Exotic PhasesDavid & Lucile Packard Foundatio
Going Beyond Counting First Authors in Author Co-citation Analysis
The present study examines one of the fundamental aspects of author co-citation analysis (ACA) - the way co-citation
counts are defined. Co-citation counting provides the data on which all subsequent statistical analyses and mappings
are based, and we compare ACA results based on two different types of co-citation counting - the traditional type that
only counts the first one among a cited work's authors on the one hand and a non-traditional type that takes into
account the first 5 authors of a cited work on the other hand. Results indicate that the picture produced through this non-traditional author co-citation counting contains more coherent author groups and is therefore considerably clearer. However, this picture represents fewer specialties in the research field being studied than that produced through the traditional first-author co-citation counting when the same number of top-ranked authors is selected and analyzed. Reasons for these effects are discussed
Homogeneous quantum gases: strongly interacting fermions and rotating bosonic condensates
Quantum gases are an ideal platform for studying problems in many-body physics. Highly tunable and reconfigurable, these systems work as quantum simulators for a range of other quantum mechanical systems, ranging from neutron stars, to superconductors, to quantum Hall systems. A crucial degree of freedom is the external geometry of the trapping potential. In this thesis, we describe experiments on creating homogeneous quantum gases and performing measurements using them.
The first section of the thesis focuses on homogeneous Fermi gases, where we use tailored optical potentials to trap 6Li atoms in a homogeneous box potential. We observe uniform fermionic superfluids and measure the temperature dependence of the noninteracting Fermi surface. Radiofrequency (rf) spectroscopy offers unique insights into the spectral properties of Fermi gases. We exploit the high signal to noise ratio of rf spectroscopy of uniform Fermi gases to obtain precise measurements of the thermodynamic contact. We observe a dramatic change in the contact at the superfluid transition.
The second section of this thesis concerns uniform rotating bosonic condensates. We discuss a new experimental apparatus and outline how geometric squeezing can be used to prepare systems of quantum gases in the lowest Landau level, a long sought-after goal. Lastly, we show a surprising spontaneous crystallization of these quantum Hall systems, and find that it is driven by interactions.Ph.D
Anomalous Translational And Reorientational Dynamics Of Single File Water
This thesis deals with several aspects of translational and reorientational dynamics of water molecules confined inside narrow carbon nanotubes. Water molecules confined in a non-polar, nanoscopic pore exhibit extremely unusual structural and dynamical properties. Adding to the list of anomalies which are already present in bulk liquid water, the confined water “chains” and “shells” springs many more surprises. The relatively weak interaction with the surrounding walls in conjuction with the strong inter-water hydrogen bonds lead o several novel structural and dynamical features, very special to this “strange” phase of water. In this thesis, we present our findings on the detailed molecular level description of translational and reorientational dynamics of this novel phase of anomalously “soft” water. Chapter 1 introduces the varied theoretical, numerical and experimental attempts to demystify the properties of bulk, interfacial and confined water. It also motivates the aspects of diffusion in low dimensional systems, which are often termed “anomalous”.
In Chapter 2, we study the structure and dynamics of water molecules inside an open ended carbon nanotube placed in a bath of water molecules. The size of the nanotube allows only a single file of water molecules inside the nanotube. The water molecules inside the nanotube show solid-like ordering at room temperature, which we quantify by calculating the pair correlation function. It is shown that even for the longest observation times, the mode of diffusion of the water molecules inside the nanotube is Fickian and not sub-diffusive. We also propose a one-dimensional random walk model for the diffusion of the water molecules inside the nanotube. We find good agreement between the mean-square displacements calculated from the random walk model and from MD simulations, thereby confirming that the water molecules undergo normal-mode diffusion inside the nanotube. We attribute this behavior to strong positional correlations that cause all the water molecules inside the nanotube to move collectively as a single object. The average residence time of the water molecules inside the nanotube is shown to scale quadratically with the nanotube length.
In Chapter 3, we study the diffusion of water molecules confined inside narrow (6,6) carbon nanorings. The water molecules form two oppositely polarised clusters. It is shown that the effective interaction between these two clusters is repulsive in nature. The computed mean-squared displacement (MSD) clearly shows a scaling with time, which is consistent with single file diffusion (SFD). The time up to which the water molecules undergo SFD is shown to be the lifetime of the water molecules inside these clusters. The inter-cluster repulsive interactions are electrostatic and hence long-ranged, which is in complete contrast with shorter ranged steric repulsion in other systems which exhibit SFD.
In Chapter 4, we study the anisotropic orientational dynamics of water molecules confined in narrow carbon nanotubes and nanorings. We find that confinement leads to strong anisotropy in the orientational relaxation. The relaxation of the aligned dipole moments, occurring on a timescale of nanoseconds, is three order of magnitude slower than that of bulk water. In contrast, the relaxation of the vector joining the two hydrogens is ten times faster compared to bulk, with a timescale of about 150 femtoseconds. The slow dipolar relaxation is mediated by the hopping of orientational defects, which are nucleated by the water molecules outside the tube, across the linear water chain.
In Chapter 5, we study the reorientational dynamics of water molecules confined inside narrow carbon nanotubes immersed in a bath of water. Our simulations show that the confined water molecules exhibit bistability in their reorientational relaxation, which proceeds by angular jumps between the two stable states. The energy barrier between these two states is about 2kBT. The effect of non-Markovian jumps shows up in the ratio of the timescales o the first and second order reorientational correlation functions, which exceeds the value of the ratio in the diffusive limit. The analytical solution of a proposed model is also presented, which qualitatively explains this “unusual” relaxation. These results will have important implications in understanding proton conduction in water-filled ion channels.
In Chapter 6, we report the thermodynamic aspects of the translational and re-orientational dynamics of the strongly confined water molecules. Considering the energetics it is surprising that the water molecules spontaneously fill up the nanotube. Thus the thermodynamics of entry of water molecules in the hydrophobic cavity of nanotube. This is generally attributed to the rotational entropy gain by the water molecules on entering the tube, a fact which has not been demonstrated quantitatively so far. We show that the gain in rotational component of the entropy compensates the loss of energy of the water molecules upon entering the nanotube.
In Chapter 7, we conclude by summarising the work done in the previous chapters and discuss the future course of actions. We would like to extend the studies on the diffusion of water inside finite nanotubes in the presence of bathwater outside, to nanotube lengths, where it is possible to observe the cross-over from an initial “single file” to and eventual, centre of mass dominated, “normal” diffusion. The mean field estimate of the length of the nanotube required so that one observes a crossover from the initial “single file” to “normal” diffusion at 100 ps is about 700
˚A. Simulation of such a system would possibly provide an unambiguous answer to the question, whether it is possible to observe SFD in finite carbon nanotubes, filled with water. Regarding the reorientational dynamics, we would like to extend our understanding of the reorientational relaxation of water chains to more more complicated structures. Depending on the diameter of the confining nanotube water molecules form polygons of ice. In the present situation each water molecule can be in only two possible states of orientation. Hence, it would be interesting to predict the reorientational dynamics for other ice structures, where each water molecule can be more “orientational states”.
In Chapter 8, we report a work which is unrelated to the rest of this thesis. The work has been done in collaboration with Prof. T. V. Ramakrishnan and Prof. Vijay
B. Shenoy. We report a novel method for the calculation of elastic constants of a solid in the frame work of Ramakrishnan-Youssouf density functional theory. The structural aspect of the liquid to solid transition and how it affects the elastic constants of the solids is brought out very clearly. The calculation is analytical and we obtain explicit expressions for the elastic constants. The description of the solid is in terms of the structure factor, S(G), of the coexisting liquid. The elastic constants are expressed as a function of equilibrium parameters, such as c(0), relatedto the compressibility of the liquid. Another important quantity on which the elastic constants depend is the curvature, c"(|G|), of c(|q|)curve at its peak (q= G). These quantities are known experimentally for many systems, and can also be calculated accurately. The shear modulus depends only on c"(|G|), while the bulk modulus has contributions from both c"(|G|) and c(0). The obtained elastic constants do not satisfy the Cauchy relations, in that C12 is not equal to C44. Calculations have been performed for two-dimensional square and triangular lattices as well as bcc and fcc lattices in three dimensions. It is seen that in order to get good agreement between the theoretical and the experimental results of the elastic constants, three body correlations have to be introduced in the calculations for the bcc and the fcc lattices. For the last, in which two shells of reciprocal lattice vectors are appropriate, we point out the modifications needed for choosing the lattice parameter in the unstrained freezing problem. We obtain a new, first principles, quasiuniversal relation for elastic constants, scaled by the melting temperature, that is experimentally satisfied. It is similar to the famous Verlet criterion that S(|G|) = 2.9 at freezing and is free of some of the unphysical aspects of previous work
Motion of a Solitonic Vortex in the BEC-BCS Crossover
We observe a long-lived solitary wave in a superfluid Fermi gas of [superscript 6]Li atoms after phase imprinting. Tomographic imaging reveals the excitation to be a solitonic vortex, oriented transverse to the long axis of the cigar-shaped atom cloud. The precessional motion of the vortex is directly observed, and its period is measured as a function of the chemical potential in the BEC-BCS crossover. The long period and the correspondingly large ratio of the inertial to the bare mass of the vortex are in good agreement with estimates based on superfluid hydrodynamics that we derive here using the known equation of state in the BEC-BCS crossover.National Science Foundation (U.S.)United States. Army Research Office. Multidisciplinary University Research Initiative on AtomtronicsUnited States. Air Force Office of Scientific Research. Presidential Early Career Award for Scientists and EngineersUnited States. Office of Naval ResearchUnited States. Defense Advanced Research Projects Agency. Optical Lattice Emulator ProgramDavid & Lucile Packard Foundatio
Variations on the Author
“Variations on the Author” discusses two of Eduardo Coutinho’s recent films (Um Dia na Vida, from 2010, and Últimas Conversas, posthumously released in 2015) and their contribution to the general question of documentary authorship. The director’s filmography is characterized by a consistent yet self-effacing form of authorial self-inscription: Coutinho often features as an interviewer that rather than express opinions propels discourses; an interviewer that is good at listening. This mode of self-inscription characterizes him as an author who is not expressive but who is nonetheless markedly present on the screen. In Um Dia na Vida, however, Coutinho is completely absent form the image, while Últimas Conversas, on the contrary, includes a confessional prologue that moves the director from the margins to the center of his films. This article examines the ways in which these works stand out in the filmography of a director who offers new insights into the notion of cinematic authorship
Appropriate Similarity Measures for Author Cocitation Analysis
We provide a number of new insights into the methodological discussion about author cocitation analysis. We first argue that the use of the Pearson correlation for measuring the similarity between authors’ cocitation profiles is not very satisfactory. We then discuss what kind of similarity measures may be used as an alternative to the Pearson correlation. We consider three similarity measures in particular. One is the well-known cosine. The other two similarity measures have not been used before in the bibliometric literature. Finally, we show by means of an example that our findings have a high practical relevance.information science;Pearson correlation;cosine;similarity measure;author cocitation analysis
Dispelling the Myths Behind First-author Citation Counts
We conducted a full-scale evaluative citation analysis study of scholars in the XML research field to explore just how different from each other author rankings resulting from different citation counting methods actually are, and to demonstrate the capability of emerging data and tools on the Web in supporting more realistic citation counting methods. Our results contest some common arguments for the continued
use of first-author citation counts in the evaluation of scholars, such as high correlations between author rankings by first-author citation counts and other citation
counting methods, and high costs of using more realistic citation counting methods that are not well-supported by the ISI databases. It is argued that increasingly available digital full text research papers make it possible for citation analysis studies to go beyond what the ISI databases have directly supported and to employ more
sophisticated methods
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