1,720,965 research outputs found
Spatially coherent high-order harmonics generated at optimal high gas pressure with high-intensity one- or two-color laser pulses
Full text linkCitation: Jin, C., & Lin, C. D. (2016). Spatially coherent high-order harmonics generated at optimal high gas pressure with high-intensity one- or two-color laser pulses. Physical Review A, 94(4), 6. doi:10.1103/PhysRevA.94.043804We investigate the gas-pressure dependence of macroscopic harmonic spectra generated in a high-ionization medium using intense 800-nm laser pulses. The harmonics obtained at the optimal pressure show good spatial coherence with small divergence (less than 2 mrad) in the far field. By analyzing the evolution of the laser's electric field as it propagates, we find that dynamic phase matching conditions are fulfilled in the second half of the gas cell and that harmonic yields do not depend on the position of the gas cell with respect to the focusing position. We also demonstrate that harmonic yields at the optimal pressure can be further enhanced by increasing input laser energy or by adding a few percent of second or third harmonic to the fundamental
Optimal generation of spatially coherent soft X-ray isolated attosecond pulses in a gas-filled waveguide using two-color synthesized laser pulses
Full text linkCitation: Jin, C., Hong, K. H., & Lin, C. D. (2016). Optimal generation of spatially coherent soft X-ray isolated attosecond pulses in a gas-filled waveguide using two-color synthesized laser pulses. Scientific Reports, 6, 11. doi:10.1038/srep38165We numerically demonstrate the generation of intense, low-divergence soft X-ray isolated attosecond pulses in a gas-filled hollow waveguide using synthesized few-cycle two-color laser waveforms. The waveform is a superposition of a fundamental and its second harmonic optimized such that highest harmonic yields are emitted from each atom. We then optimize the gas pressure and the length and radius of the waveguide such that bright coherent high-order harmonics with angular divergence smaller than 1 mrad are generated, for photon energy from the extreme ultraviolet to soft X-rays. By selecting a proper spectral range enhanced isolated attosecond pulses are generated. We study how dynamic phase matching caused by the interplay among waveguide mode, neutral atomic dispersion, and plasma effect is achieved at the optimal macroscopic conditions, by performing time-frequency analysis and by analyzing the evolution of the driving laser's electric field during the propagation. Our results, when combined with the on-going push of high-repetition-rate lasers (sub- to few MHz's) may eventually lead to the generation of high-flux, low-divergence soft X-ray tabletop isolated attosecond pulses for applications
Analysis of THz generation through the asymmetry of photoelectron angular distributions
Full text linkCitation: Zhou, Z. Y., Wang, X., & Lin, C. D. (2017). Analysis of THz generation through the asymmetry of photoelectron angular distributions. Physical Review A, 95(3), 6. doi:10.1103/PhysRevA.95.033418We analyze the mechanism of THz generation in a gas medium with intense two-color infrared lasers pulses. The dependence of the amplitude of THz emission on the relative phase between the fundamental color (800 nm) and its second harmonic (400 nm) is shown to be identical to the residual current as well as to the asymmetry of the above-threshold-ionization (ATI) photoelectrons along the left versus the right side of the linear polarization axis of the laser, thus confirming the validity of the semiclassical photocurrent model for the THz emission. We further analyze the even vs odd angular momentum distributions of the ATI electrons. The degree of overlap between the even-parity dominant electrons and the odd-parity dominant electrons within each ATI peak determines the strength of the THz emission, thus favoring the model that THz is generated through free-free transitions in the laser field. A model is also provided to obtain the same phase dependence as the four-wave mixing model
Phase-retrieval algorithm for the characterization of broadband single attosecond pulses
Full text linkCitation: Zhao, X., Wei, H., Wu, Y., & Lin, C. D. (2017). Phase-retrieval algorithm for the characterization of broadband single attosecond pulses. Physical Review A, 95(4), 8. doi:10.1103/PhysRevA.95.043407Recent progress in high-order harmonic generation with few-cycle mid-infrared wavelength lasers has pushed light pulses into the water-window region and beyond. These pulses have the bandwidth to support single attosecond pulses down to a few tens of attoseconds. However, the present available techniques for attosecond pulse measurement are not applicable to such pulses. Here we report a phase-retrieval method using the standard photoelectron streaking technique where an attosecond pulse is converted into its electron replica through photoionization of atoms in the presence of a time-delayed infrared laser. The iterative algorithm allows accurate reconstruction of the spectral phase of light pulses, from the extreme-ultraviolet (XUV) to soft x-rays, with pulse durations from hundreds down to a few tens of attoseconds. At the same time, the streaking laser fields, including short pulses that span a few octaves, can also be accurately retrieved. Such well-characterized single attosecond pulses in the XUV to the soft-x-ray region are required for time-resolved probing of inner-shell electronic dynamics of matter at their own timescale of a few tens of attoseconds
Retrieval of target structure information from laser-induced photoelectrons by few-cycle bicircular laser fields
Full text linkCitation: Hoang, V. H., Le, V. H., Lin, C. D., & Le, A. T. (2017). Retrieval of target structure information from laser-induced photoelectrons by few-cycle bicircular laser fields. Physical Review A, 95(3), 6. doi:10.1103/PhysRevA.95.031402By analyzing theoretical results from a numerical solution of the time-dependent Schrodinger equation for atoms in few-cycle bicircular laser pulses, we show that high-energy photoelectron momentum spectra can be used to extract accurate elastic scattering differential cross sections of the target ion with free electrons. We find that the retrieval range for a scattering angle with bicircular pulses is wider than with linearly polarized pulses, although the retrieval method has to be modified to account for different returning directions of the electron in the continuum. This result can be used to extend the range of applicability of ultrafast imaging techniques such as laser-induced electron diffraction and for the accurate characterization of laser pulses
Probing and extracting the structure of vibrating SF6 molecules with inner-shell photoelectrons
Full text linkCitation: Nguyen, N. T., Lucchese, R. R., Lin, C. D., & Le, A. T. (2016). Probing and extracting the structure of vibrating SF6 molecules with inner-shell photoelectrons. Physical Review A, 93(6), 9. doi:10.1103/PhysRevA.93.063419We propose a scheme for probing the structure of vibrating molecules with photoelectrons generated from ultrashort soft-x-ray pulses. As an example we analyze below-100-eV photoelectrons liberated from the S(2p) orbital of vibrating SF6 molecules to image very small structural changes of molecular vibration. In particular, photoionization cross sections and photoelectron angular distributions (PAD) at nonequilibrium geometries can be retrieved accurately with photoelectrons near the shape resonance at 13 eV. This is achieved with a pump-probe scheme, in which the symmetric stretch mode is first Raman excited predominantly by a relatively short laser pulse and then later probed at different time delays by a few-femtosecond soft-x-ray pulse with photon energy near 200 eV
Influence of orbital symmetry on diffraction imaging with rescattering electron wave packets
Full text linkCitation: Pullen, M. G., Wolter, B., Le, A. T., Baudisch, M., Sclafani, M., Pires, H., . . . Biegert, J. (2016). Influence of orbital symmetry on diffraction imaging with rescattering electron wave packets. Nature Communications, 7, 6. doi:10.1038/ncomms11922The ability to directly follow and time-resolve the rearrangement of the nuclei within molecules is a frontier of science that requires atomic spatial and few-femtosecond temporal resolutions. While laser-induced electron diffraction can meet these requirements, it was recently concluded that molecules with particular orbital symmetries (such as pi(g)) cannot be imaged using purely backscattering electron wave packets without molecular alignment. Here, we demonstrate, in direct contradiction to these findings, that the orientation and shape of molecular orbitals presents no impediment for retrieving molecular structure with adequate sampling of the momentum transfer space. We overcome previous issues by showcasing retrieval of the structure of randomly oriented O-2 and C2H2 molecules, with pi(g) and pi(u) symmetries, respectively, and where their ionization probabilities do not maximize along their molecular axes. While this removes a serious bottleneck for laser-induced diffraction imaging, we find unexpectedly strong backscattering contributions from low-Z atoms
Going Beyond Counting First Authors in Author Co-citation Analysis
Full text linkThe present study examines one of the fundamental aspects of author co-citation analysis (ACA) - the way co-citation
counts are defined. Co-citation counting provides the data on which all subsequent statistical analyses and mappings
are based, and we compare ACA results based on two different types of co-citation counting - the traditional type that
only counts the first one among a cited work's authors on the one hand and a non-traditional type that takes into
account the first 5 authors of a cited work on the other hand. Results indicate that the picture produced through this non-traditional author co-citation counting contains more coherent author groups and is therefore considerably clearer. However, this picture represents fewer specialties in the research field being studied than that produced through the traditional first-author co-citation counting when the same number of top-ranked authors is selected and analyzed. Reasons for these effects are discussed
Variations on the Author
Full text link“Variations on the Author” discusses two of Eduardo Coutinho’s recent films (Um Dia na Vida, from 2010, and Últimas Conversas, posthumously released in 2015) and their contribution to the general question of documentary authorship. The director’s filmography is characterized by a consistent yet self-effacing form of authorial self-inscription: Coutinho often features as an interviewer that rather than express opinions propels discourses; an interviewer that is good at listening. This mode of self-inscription characterizes him as an author who is not expressive but who is nonetheless markedly present on the screen. In Um Dia na Vida, however, Coutinho is completely absent form the image, while Últimas Conversas, on the contrary, includes a confessional prologue that moves the director from the margins to the center of his films. This article examines the ways in which these works stand out in the filmography of a director who offers new insights into the notion of cinematic authorship
- …
