61 research outputs found
Dressed projectile charge state dependence of differential electron emission from Ne atom
No full textWe study the projectile charge state dependence of doubly differential electron emission cross section (DDCS) in ionization of Ne under the impact of dressed and bare oxygen ions. Experimental DDCS results measured at different angles are compared with the calculations based on a CDW-EIS approximation using the GSZ model potential to describe projectile active-electron interaction. This prescription gives an overall very good agreement. In general a deviation from the q2-law was observed in the DDCS. The observations crudely identify the dominance of different projectile electron loss mechanisms at certain electron energy range.Fil: Biswas, S.. Tata Institute of Fundamental Research; IndiaFil: Monti, Juan Manuel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Rivarola, Roberto Daniel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Tribedi, L. C.. Tata Institute of Fundamental Research; Indi
Ionization Dynamics in Fast Ion-Atom Collisions. II. Final-State Momentum Distributions of the Ionization Products in Collisions of He with Bare Carbon Ions
No full textWe have used the energy and angular distributions of the low-energy electron emission cross sections from the preceding paper [Lokesh C. Tribedi et al., Phys. Rev. A 58, 3619 (1998)] to derive the doubly differential final-state longitudinal momentum distributions of the electrons, recoil ions, and projectiles in ion-atom ionization for [Formula Presented] The complementary nature of the electron spectroscopy and the recoil-ion momentum spectroscopy have been investigated using a formulation based on three-body kinematics to explore the ionization dynamics in detail. The influence of the three-body ionization as well as the binary-encounter processes on the recoil-ion (and projectile) longitudinal momentum distributions has been investigated. The separation of the soft- and hard-collision branches of recoil-ion distributions is an important feature of the present technique. The present method also allows one to determine cross sections for very large electron momenta. The single- differential distributions are also derived by numerical integration of the double-differential distributions. The first Born approximation, the continuum distorted wave eikonal initial state, and the classical trajectory Monte Carlo calculations are used to explain the data. © 1998 The American Physical Society
Ionization Dynamics in Fast Ion-Atom Collisions. I. Energy and Angular Distributions of Low-Energy Electrons Emitted in Ionization of He by Bare Carbon Ions
No full textWe have studied the two-center effect (TCE) in ion-atom ionization by measuring the energy and angular distributions of the double-differential cross sections (DDCSs) (d2σ/dεdΩ) of the low-energy electrons emitted in a collision of He atoms with 2.5 MeV/nucleon C6+ ions. The electrons with energies between 0.1 and 300 eV were detected for 13 different emission angles between 15° and 160°. From the measured DDCSs we have deduced the single differential cross sections such as dσ/dΩ and dσ/dε and the total cross section. The data have been compared with the continuum distorted wave eikonal initial state calculations with H-like and Hartree-Fock-Slater wave functions for the initial and final state of the electron and first Born calculations. The forward-backward asymmetry parameter also has been deduced to study the TCE in detail. In the following paper [Lokesh C. Tribedi et al., Phys. Rev. A 58, 3626 (1998)] we have explored the collision dynamics by deducing the momentum distributions of the electron, the recoil ion, and the projectile
Energy and angular distribution of electrons in ionization of He and Ne by 6-MeV/u bare carbon ions: Comparison with continuum-distorted-wave eikonal-initial-state calculations in prior and post forms
No full textWe have measured the absolute double-differential cross sections (DDCS) for electron emission in ionization of He and Ne atoms under the impact of 6-MeV/u C6+ ions. Data were collected between 1 and 500 eV for He, while for Ne this range was extended up to 1000 eV. The angular ranges covered in the experiment are 30∘ to 150∘ and 20∘ to 160∘ for He and Ne, respectively. The DDCS spectra are compared with the prior and the post forms of the state-of-the-art continuum-distorted-wave eikonal-initial-state model. Both the theoretical models show very good agreement with the energy and angular distributions of the DDCS in the case of He. For Ne, at low energies both are going together and matching very well with the data. In the high-energy region, at extreme forward and backward angles, although both the forms are underestimating the experimental data to some extent, the prior form shows much better agreement compared to the post form. This post-prior discrepancy is attributed to the influence of dynamic screening, on the ionized one, produced by the electrons remaining in the target. The single differential cross sections (SDCS) in emission angle (dσdΩe) and electron energy (dσdεe) are deduced by integrating the electron DDCS spectra. While excellent agreement is obtained for the dσdεe spectrum, the dσdΩe provides a further sensitive test to the adequacy of the theoretical model employed. The total cross section obtained from the SDCS spectra is about 11% higher than the prior model for He and about 6% lower for Ne. To get the quantitative picture of the two-center effect, the forward-backward angular asymmetry parameter has been deduced as a function of velocity of the ejected electrons. For both the targets, it is very well reproduced by both the forms of the theory. For the Ne target, K-LL Auger angular distribution has also been studied, which shows small asymmetry caused by multiple vacancies in the L shell along with the K-shell vacancy.Fil: Biswas, Shubhadeep. International Centre Of Theoretical Science. Tata Institute Of Fundamental Research; EspañaFil: Misra, D.. International Centre Of Theoretical Science. Tata Institute Of Fundamental Research; EspañaFil: Monti, Juan Manuel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Rosario. Instituto de Física de Rosario (i); ArgentinaFil: Tachino, Carmen Alejandra. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Rosario. Instituto de Física de Rosario (i); ArgentinaFil: Rivarola, Roberto Daniel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Rosario. Instituto de Física de Rosario (i); ArgentinaFil: Tribedi, L. C.. International Centre Of Theoretical Science. Tata Institute Of Fundamental Research; Españ
Double-differential cross sections for ionization of H2O by fast bare O ions: Comparison with continuum-distorted-wave eikonal-initial-state calculations in prior and post forms
No full textO vapor in a static gas condition which allowed us to deduce the absolute value of the cross sections. The single-differential cross sections (SDCS) and the total cross sections have also been obtained. The DDCS as well as the SDCS spectra are compared with the continuum-distorted-wave eikonal-initial-state (CDW-EIS) calculations for both the prior as well as the post forms of the scattering matrix. The initial state is represented within the complete neglect of differential overlap approximation, where the molecular orbitals are expressed in terms of atomic orbitals of the atomic constituents. The overall agreement with the CDW-EIS model is quite good as far as the energy dependence is concerned. The prior form of the model is found to provide a better understanding of the data compared to the post version. In particular, excellent agreement between the theory and experiment has been observed for the angular distribution data at forward angles.Fil: Nandi, S.. International Centre Of Theoretical Science. Tata Institute Of Fundamental Research; EspañaFil: Biswas, S.. International Centre Of Theoretical Science. Tata Institute Of Fundamental Research; EspañaFil: Khan, A.. International Centre Of Theoretical Science. Tata Institute Of Fundamental Research; EspañaFil: Monti, Juan Manuel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Rosario. Instituto de Física de Rosario (i); ArgentinaFil: Tachino, Carmen Alejandra. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Rosario. Instituto de Física de Rosario (i); ArgentinaFil: Rivarola, Roberto Daniel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Rosario. Instituto de Física de Rosario (i); ArgentinaFil: Misra, D.. International Centre Of Theoretical Science. Tata Institute Of Fundamental Research; EspañaFil: Tribedi, L. C.. International Centre Of Theoretical Science. Tata Institute Of Fundamental Research; Españ
Electron emission in fast heavy ion impact ionization of C
No full textWe have measured the energy and angle differential ejected electron spectra of C60 as well as Ne atoms in collisions with 4 MeV/u bare fluorine projectile ions. Absolute cross sections have been estimated for electron emission in the energy range of 1 eV–300 eV, including the KLL-Auger electrons for various angles between 30° and 150°. The double differential cross sections for C60 have been compared with the state-of-the-art CDW-EIS model under CNDO approximation as well as with the data for the Ne target. The C60 spectra at all angles show a broad giant plasmon resonance in the low energy region, which is not present in the atomic target data. The angular distribution reveals the dipolar nature of the plasmon excitation. The C K-LL Auger emission from C60 reveals a large angular anisotropy compared to that for a hydrocarbon, e.g. methane target
Differential electron emission in the ionization of Ne and Xe atoms under fast bare carbon ion impact
No full textMeasurement of the energy and angular distributions of the double differential cross section (DDCS) of electron emission from Ne and Xe atoms in collision with 5 MeV u-1 bare carbon ions is reported. This study aimed to investigate the electron emission processes in the case of multi-electronic systems. In general, several clear differences between the electron emission spectra of Ne and Xe are found, which indicate the influence of the increasing number of electrons. For instance, the sharp peak due to the binary nature of collision is almost absent in the case of Xe, unlike Ne, which could be understood due to the increasing contribution from the strongly bound inner shell (such as) electrons for the Xe atom. The forward-backward angular asymmetry has also been derived from the angular distributions. For Xe, the qualitative behaviour of the asymmetry parameter is seen to be quite different since it reveals structures due to Auger contributions. It is, in general, different and much lower than that for Ne, which shows the smooth behaviour that one finds for other lighter atoms like He. The single differential and total cross sections are also derived. The theoretical calculations based on the prior form of the continuum distorted wave-eikonal initial state (CDW-EIS) approximation have been provided for both the targets. Overall, it gives a very good agreement with the energy and the angular distributions of DDCS for Ne. For Xe, the agreement is not as good as for Ne. We also provide a detailed discussion on the DDCS obtained from different sub-shell ionization, estimated in this framework.Fil: Biswas, Shubhadeep. International Centre Of Theoretical Science. Tata Institute Of Fundamental Research; EspañaFil: Monti, Juan Manuel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Tachino, Carmen Alejandra. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Rivarola, Roberto Daniel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Tribedi, L. C.. International Centre Of Theoretical Science. Tata Institute Of Fundamental Research; Españ
Angular momentum sensitive two-center interference
No full textIn quantum mechanics the Young-type double-slit experiment can be performed with electrons either traveling through a double slit or being coherently emitted from two inversion symmetric molecular sites. In the latter one the valence photoionization cross sections of homonuclear diatomic molecules were predicted to oscillate over kinetic energy almost 50 years ago. Beyond the direct proof of the oscillatory behavior of these photoionization cross sections σ, we show that the angular distribution of the emitted electrons reveals hitherto unexplored information on the relative phase shift between the corresponding partial waves through two-center interference patterns
Absolute total ionization cross sections of uracil (C4H4N2O2) in collisions with MeV energy highly charged carbon, oxygen and fluorine ions
No full textIonization and fragmentation of uracil molecules (C4H4N2O2, m = 112 amu) in collisions with fast highly charged C, O and F ions have been investigated using a time-of-flight mass spectrometer. The measurement of total ionization cross sections (TCS) is reported for different charge states (q), such as Fq + with q = 5–8; Oq + with q = 5,7; Cq + with q = 5 and 6. These studies reveal a (q/v)~1.5 dependence of TCS, in contrast, to the well-known q2-dependence in ion–atom collisions. Scaling properties of the TCS with projectile energy and charge states are obtained. The experimental results for TCS measurements are compared with the theoretical calculations performed within classical and quantum mechanical frameworks. The trends in energy dependence of the TCSs is qualitatively well reproduced by the different models and more specifically by the classical description, which provides the best agreement with measurements.Fil: Agnihotri, A. N.. International Centre Of Theoretical Science. Tata Institute Of Fundamental Research; EspañaFil: Kasthurirangan, S. Institute of Chemical Technology; IndiaFil: Nandi, S.. International Centre Of Theoretical Science. Tata Institute Of Fundamental Research; EspañaFil: Kumar, A.. BARC. Nuclear Physics Division; IndiaFil: Champion, C.. Universite Paul Verlaine-metz; FranciaFil: Lekadir, H.. Universite Paul Verlaine-metz; FranciaFil: Hanssen, Jocelyn. Universite Paul Verlaine-metz; FranciaFil: Weck, P. F.. University of Nevada. Department of Chemistry; Estados UnidosFil: Galassi, Mariel Elisa. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Rosario. Instituto de Física de Rosario (i); ArgentinaFil: Rivarola, Roberto Daniel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Rosario. Instituto de Física de Rosario (i); ArgentinaFil: Fojon, Omar Ariel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Rosario. Instituto de Física de Rosario (i); ArgentinaFil: Tribedi, L.. International Centre Of Theoretical Science. Tata Institute Of Fundamental Research; Españ
L-MM Auger electron emission from chlorinated organic molecules under proton impact: angular distribution and total cross section measurement
No full textWe have measured absolute total cross section for LMM Auger electron emission
of Cl in chlorinated methane and benzene chloride in collision with H+ ion.
Projectile energy dependence of the total yield as well as the angular
distribution has been studied. Incident proton energy has been varied from 125
keV to 275 keV in steps of 50 keV. C KLL Auger yield have been compared with
previous studies and found to be in agreement within the effect of chemical
species It has been found that the LMM Auger yield of Cl is much more
significantly affected by molecular environment than the C KLL
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