DIFFER: Publications
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Benchmarking of Monte Carlo Flux simulations of electrons in CO2
Electron velocity distribution functions (EVDFs) in CO2 obtained by means of the Monte Carlo Flux (MCF) method are compared with results from two-term and multi-term Boltzmann solvers. The MCF method provides detailed calculations of the EVDF through a highly efficient variance reduction technique. Benchmark calculations of Legendre polynomial coefficients of the EVDF expansion are reported for a wide range of reduced electric fields (E/N), showing excellent agreement with multi-term solutions. Rate coefficients of inelastic processes calculated from two-term Boltzmann solvers differ significantly, up to 70%, from MCF and multi-term solutions, due to the anisotropy of the EVDF. An extension of the method to consider the thermal distribution of the background gas is also presented. This extension, together with an accurate description of the population of rotationally and vibrationally excited states, provides excellent agreement with measured transport coefficients at low E/N. A good agreement is obtained at moderate E/N between experimental values of dissociation rate coefficients and MCF calculations after careful consideration and analysis of several cross sections data sets.</p
Numerical Study of Jet-Target Interaction: Influence of Dielectric Permittivity on the Electric Field Experienced by the Target
This work presents a study of the influence of dielectric permittivity on the interaction between a positive pulsed He plasma jet and a 0.5 mm-thick dielectric target, using a validated two-dimensional numerical model. Six different targets are studied: five targets at floating potential with relative permittivities ϵr= 1, 4, 20, 56 and 80; and one grounded target of permittivity ϵr=56. The temporal evolution of the charging of the target and of the electric field inside the target are described, during the pulse of applied voltage and after its fall. It is found that the order of magnitude of the electric field inside the dielectric targets is the same for all floating targets with ϵr≥4. For all these targets, during the pulse of applied voltage, the electric field perpendicular to the target and averaged through the target thickness, at the point of discharge impact, is between 1 and 5 kV cm−1. For the two remaining targets (ϵr=1 and grounded target with ϵr=56), the field is significantly higher than for all the other floating targets.</p
Core tungsten transport in WEST long pulse L-mode plasmas
Tungsten transport is investigated in WEST long pulse L-mode plasmas operated with the strike point on the actively cooled upper tungsten divertor. The pulses are mostly heated by lower hybrid waves. It is experimentally found that tungsten does not centrally accumulate throughout these similar to 30 s reproducible discharges despite large normalised electron density gradients R/L-ne. To explain these observations, turbulent and neoclassical transport of electrons and tungsten ions are computed with GKW Peeters A.G. et al (2009 Computer Phys. Commnun. 180 2650) and NEO Belli E. and Candy J. (2008 Plasma Phys. Control. Fusion 50 095010), Belli E. and Candy J. (2012 Plasma Phys. Control. Fusion 54 015015) respectively. Additionally, interpretative integrated modelling simulations are also performed to keep data coherency despite the lack of measurements of some quantities such as the Ti profiles. Modelled R/Lne are found consistent with interferometry inversions and the tungsten peaking factor R/L-nW remains comparable to R/L-ne due to dominant turbulent diffusivities inside r/a = 0.3-0.8. In the central region r/a < 0.3 neoclassical W transport dominates but the convective velocities are several order of magnitudes lower compared to plasmas with toroidal rotation velocities induced by a neutral beam injection (NBI) torque. Finally, nitrogen is seeded in these pulses leading to an enhanced energy content which is consistent with stabilised ion temperature gradient modes from dilution
Runaway electron synchrotron radiation in a vertically translated plasma
Synchrotron radiation observed from runaway electrons (REs) in tokamaks depends upon the position and size of the RE beam, the RE energy and pitch distributions, as well as the location of the observer. We show experimental synchrotron images of a vertically moving RE beam sweeping past the detector in the Tokamak à Configuration Variable (TCV) tokamak and compare it with predictions from the synthetic synchrotron diagnostic Soft. This experimental validation lends confidence to the theory underlying the synthetic diagnostics which are used for benchmarking theoretical models of and probing runaway dynamics. We present a comparison of synchrotron measurements in TCV with predictions of kinetic theory for runaway dynamics in uniform magnetic fields. We find that to explain the detected synchrotron emission, significant non-collisional pitch angle scattering as well as radial transport of REs would be needed. Such effects could be caused by the presence of magnetic perturbations, which should be further investigated in future TCV experiments
Isotope dependence of energy, momentum and particle confinement in tokamaks
The isotope dependence of plasma transport will have a significant impact on the performance of future D-T experiments in JET and ITER and eventually on the fusion gain and economics of future reactors. In preparation for future D-T operation on JET, dedicated experiments and comprehensive transport analyses were performed in H, D and H-D mixed plasmas. The analysis of the data has demonstrated an unexpectedly strong and favourable dependence of the global confinement of energy, momentum and particles in ELMy H-mode plasmas on the atomic mass of the main ion species, the energy confinement time scaling as tau(E) similar to A(0.5) (Maggi et al., Plasma Phys. Control. Fusion, vol. 60, 2018, 014045; JET Team, Nucl. Fusion, vol. 39, 1999, pp. 1227-1244), i.e. opposite to the expectations based only on local gyro-Bohm (GB) scaling, tau(E) similar to A(-0.5), and stronger than in the commonly used H-mode scaling for the energy confinement (Saibene et al., Nucl. Fusion, vol. 39, 1999, 1133; ITER Physics Basis, Nucl. Fusion, vol. 39, 1999, 2175). The scaling of momentum transport and particle confinement with isotope mass is very similar to that of energy transport. Nonlinear local GENE gyrokinetic analysis shows that the observed anti-GB heat flux is accounted for if collisions, ExB shear and plasma dilution with low-Z impurities (Be-9) are included in the analysis (E and B are, respectively the electric and magnetic fields). For L-mode plasmas a weaker positive isotope scaling tau(E) similar to A(0.14) has been found in JET (Maggi et al., Plasma Phys. Control. Fusion, vol. 60, 2018, 014045), similar to ITER97-L scaling (Kaye et al., Nucl. Fusion, vol. 37, 1997, 1303). Flux-driven quasi-linear gyrofluid calculations using JETTO-TGLF in L-mode show that local GB scaling is not followed when stiff transport (as is generally the case for ion temperature gradient modes) is combined with an imposed boundary condition taken from the experiment, in this case predicting no isotope dependence. A dimensionless identity plasma pair in hydrogen and deuterium L-mode plasmas has demonstrated scale invariance, confirming that core transport physics is governed, as expected, by the 4 dimensionless parameters rho*, nu*, beta, q (normalised ion Larmor radius, collisionality, plasma pressure and safety factor) consistently with global quasi-linear gyrokinetic TGLF calculations (Maggi et al., Nucl. Fusion, vol. 59, 2019, 076028). We compare findings in JET with those in different devices and discuss the possible reasons for the different isotope scalings reported from different devices. The diversity of observations suggests that the differences may result not only from differences affecting the core, e.g. heating schemes, but are to a large part due to differences in device-specific edge and wall conditions, pointing to the importance of better understanding and controlling pedestal and edge processes
Robust impurity detection and tracking for tokamaks
A robust impurity detection and tracking code, able to generate large sets of dust tracks from tokamak camera footage, is presented. This machine learning–based code is tested with cameras from the Joint European Torus, Doublet-III-D, and Magnum-PSI and is able to generate dust tracks with a 65–100% classification accuracy. Moreover, the number dust particles detected from a single camera shot can be up to the order of 1000. Several areas of improvement for the code are highlighted, such as generating more significant training data sets and accounting for selection biases. Although the code is tested with dust in single two-dimensional camera views, it could easily be applied to multiple-camera stereoscopic reconstruction or nondust impurities.</p
Single Particle Approaches to Plasmon-Driven Catalysis
Plasmonic nanoparticles have recently emerged as a promising platform for photocatalysis thanks to their ability to efficiently harvest and convert light into highly energetic charge carriers and heat. The catalytic properties of metallic nanoparticles, however, are typically measured in ensemble experiments. These measurements, while providing statistically significant information, often mask the intrinsic heterogeneity of the catalyst particles and their individual dynamic behavior. For this reason, single particle approaches are now emerging as a powerful tool to unveil the structure-function relationship of plasmonic nanocatalysts. In this Perspective, we highlight two such techniques based on far-field optical microscopy: surface-enhanced Raman spectroscopy and super-resolution fluorescence microscopy. We first discuss their working principles and then show how they are applied to the in-situ study of catalysis and photocatalysis on single plasmonic nanoparticles. To conclude, we provide our vision on how these techniques can be further applied to tackle current open questions in the field of plasmonic chemistry
Response of yttria dispersion strengthened tungsten simultaneously exposed to steady-state and transient hydrogen plasma
W–Y2O3 alloy with low DBTT (ductile-brittle transition temperature) and high RCT (recrystallization temperature), processed by high energy rate forging (HERF) was exposed to ITER-like steady-state and transient hydrogen plasma in the linear plasma generator Magnum-PSI. The steady-state heat fluxes were in the range of 8.35–16.32 MW . m−2, resulting in surface base temperatures of the samples in the range of 1271 °C to 1982 °C. The applied transient peak heat flux with a frequency of 5 Hz (a total of 1000 pulses) was about 0.50 GW . m−2. The exposure time was ~220 s. No obvious morphological change of the exposed sample with a base temperature of 1271 °C was observed, except the preferential erosion of the W/Y2O3 interface. However, cracks along grain boundaries were formed on the surface of the exposed samples with base temperatures above 1389 °C. Pronounced recrystallization and grain growth also occurred for the samples with base temperatures of 1666 °C and 1982 °C. It is desirable to find that no wide and deep crack with preferential propagation direction with regard to the sample dimension was observed, even extensive recrystallization and cracking along grain boundaries occurred. This indicates that decreasing DBTT and increasing RCT simultaneously is desirable to broaden the safe operational temperature window of W as plasma-facing material, and therefore to increase the power handling capability of the plasma-facing units of a tungsten-based divertor in future fusion reactors. However, the formation of W/Y2O3 composite, melting and depletion of the Y2O3 particles gradually occurred with increasing the surface temperatures. It implies that the doping of Y2O3 particles complicates the plasma-material interaction, compared to the pure W case. For example, it raises concerns about the formation of complex dust which will potentially be a significant issue for the safe operation of future fusion reactors (e.g. core plasma contamination and fuel recycling)