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Revised assessment of local air quality in Stavanger
No full textTiltaksutredningen for lokal luftkvalitet i Stavanger, med handlingsplan og tiltak, skal bidra til at forurensningsnivået holder seg innenfor kravene i forurensningsforskriften. I tillegg belyser denne utredningen tiltak som vil være med på å redusere nivåene sammenlignet med helsemyndighetenes anbefaling til luftkvalitet. Tiltaksutredningen omfatter en kartlegging av luftkvaliteten i Stavanger ved trafikkberegninger og utslipps- og spredningsberegninger for PM10, PM2,5 og NO2 for Dagens situasjon 2018 og Framtidig situasjon 2024 med og uten tiltak. Basert på resultatene fra beregningene og i samarbeid med oppdragsgiver, er det foreslått en revidert handlings- og beredskapsplan som skal behandles politisk.The air quality assessment for Stavanger covers mapping of the air quality in Stavanger through traffic, emission and dispersion calculations of PM10, PM2,5 and NO2 for the present situation (2018) and future scenarios (2024) with and without measures. Based on the calculations and in coordination with Stavanger municipality, a plan for improved local air quality and a management plan for periods with high concentration levels is proposed for political processing.publishedVersio
Uncovering transport, deposition and impact of radionuclides released after the early spring 2020 wildfires in the Chernobyl Exclusion Zone
Get PDFIn the beginning of April 2020, large fires that started in the Chernobyl Exclusion Zone (CEZ) established after the Chernobyl accident in 1986 caused media and public concerns about the health impact from the resuspended radioactivity. In this paper, the emissions of previously deposited radionuclides from these fires are assessed and their dispersion and impact on the population is examined relying on the most recent data on radioactive contamination and emission factors combined with satellite observations. About 341 GBq of 137Cs, 51 GBq of 90Sr, 2 GBq of 238Pu, 33 MBq of 239Pu, 66 MBq of 240Pu and 504 MBq of 241Am were released in 1st–22nd April 2020 or about 1,000,000,000 times lower than the original accident in 1986 and mostly distributed in Central and East Europe. The large size of biomass burning particles carrying radionuclides prevents long-range transport as confirmed by concentrations reported in Europe. The highest cumulative effective doses (> 15 μSv) were calculated for firefighters and the population living in the CEZ, while doses were much lower in Kiev (2–5 μSv) and negligible in Belarus, Russia and Europe. All doses are radiologically insignificant and no health impact opublishedVersio
On the tuning of atmospheric inverse methods: comparisons with the European Tracer Experiment (ETEX) and Chernobyl datasets using the atmospheric transport model FLEXPART
Get PDFEstimation of the temporal profile of an atmospheric release, also called the source term, is an important problem in environmental sciences. The problem can be formalized as a linear inverse problem wherein the unknown source term is optimized to minimize the difference between the measurements and the corresponding model predictions. The problem is typically ill-posed due to low sensor coverage of a release and due to uncertainties, e.g., in measurements or atmospheric transport modeling; hence, all state-of-the-art methods are based on some form of regularization of the problem using additional information. We consider two kinds of additional information: the prior source term, also known as the first guess, and regularization parameters for the shape of the source term. While the first guess is based on information independent of the measurements, such as the physics of the potential release or previous estimations, the regularization parameters are often selected by the designers of the optimization procedure. In this paper, we provide a sensitivity study of two inverse methodologies on the choice of the prior source term and regularization parameters of the methods. The sensitivity is studied in two cases: data from the European Tracer Experiment (ETEX) using FLEXPART v8.1 and the caesium-134 and caesium-137 dataset from the Chernobyl accident using FLEXPART v10.3.publishedVersio
The presence, emission and partitioning behavior of polychlorinated biphenyls in waste, leachate and aerosols from Norwegian waste-handling facilities
Get PDFEven though production and open use of polychlorinated biphenyls (PCBs) have been phased out in Western industrialised countries since the 1980s, PCBs were still present in waste collected from different waste handling facilities in Norway in 2013. Sums of seven indicator-PCBs (I-PCB7: PCB-28, -52, -101, -118, -138, -153 and -180) were highest in plastic waste (3700 ±1800 μg/kg, n=15), waste electrical and electronic equipment (WEEE) (1300 ± 400 μg/kg, n=12) and fine vehicle fluff (1800 ± 1400 μg/kg, n=4) and lowest in glass waste, combustibles, bottom ash and fly ash (0.3 to 65 μg/kg). Concentrations in leachate water varied from 1.7 to 2900 ng/L, with higher concentrations found at vehicle and WEEE handling facilities. Particles in leachate water exhibited similar PCB sorption properties as solid waste collected on site, with waste-water partitioning coefficients ranging from 105 to 107. I-PCB7 in air samples collected at the sites were mostly in the gas phase (100–24000 pg/m3), compared to those associated with particles (9–1900 pg/m3). In contrast brominated flame retardants (BFRs) in the same samples were predominantly found associated with particles (e.g. sum of 10 brominated diethyl ethers, ΣBDE10, associated with particles 77–194,000 pg/m3) compared to the gas phase (ΣBDE10 6–473 pg/m3). Measured gas-phase I-PCB7 concentrations are less than predicted, assuming waste-air partitioning in equilibrium with predominant waste on site. However, the gas-particle partitioning behavior of PCBs and BFRs could be predicted using an established partitioning model for ambient aerosols. PCB emissions from Norwegian waste handling facilities occurred primarily in the form of atmospheric vapor or leachate particles.publishedVersio
The regional European atmospheric transport inversion comparison, EUROCOM: first results on European-wide terrestrial carbon fluxes for the period 2006–2015
Get PDFAtmospheric inversions have been used for the past two decades to derive large-scale constraints on the sources and sinks of CO2 into the atmosphere. The development of dense in situ surface observation networks, such as ICOS in Europe, enables in theory inversions at a resolution close to the country scale in Europe. This has led to the development of many regional inversion systems capable of assimilating these high-resolution data, in Europe and elsewhere. The EUROCOM (European atmospheric transport inversion comparison) project is a collaboration between seven European research institutes, which aims at producing a collective assessment of the net carbon flux between the terrestrial ecosystems and the atmosphere in Europe for the period 2006–2015. It aims in particular at investigating the capacity of the inversions to deliver consistent flux estimates from the country scale up to the continental scale. The project participants were provided with a common database of in situ-observed CO2 concentrations (including the observation sites that are now part of the ICOS network) and were tasked with providing their best estimate of the net terrestrial carbon flux for that period, and for a large domain covering the entire European Union. The inversion systems differ by the transport model, the inversion approach, and the choice of observation and prior constraints, enabling us to widely explore the space of uncertainties. This paper describes the intercomparison protocol and the participating systems, and it presents the first results from a reference set of inversions, at the continental scale and in four large regions. At the continental scale, the regional inversions support the assumption that European ecosystems are a relatively small sink (−0.21±0.2 Pg C yr−1). We find that the convergence of the regional inversions at this scale is not better than that obtained in state-of-the-art global inversions. However, more robust results are obtained for sub-regions within Europe, and in these areas with dense observational coverage, the objective of delivering robust country-scale flux estimates appears achievable in the near future.publishedVersio
Genotoxicity of Nanomaterials: Advanced In Vitro Models and High Throughput Methods for Human Hazard Assessment - A Review
Get PDFChanges in the genetic material can lead to serious human health defects, as mutations in somatic cells may cause cancer and can contribute to other chronic diseases. Genotoxic events can appear at both the DNA, chromosomal or (during mitosis) whole genome level. The study of mechanisms leading to genotoxicity is crucially important, as well as the detection of potentially genotoxic compounds. We consider the current state of the art and describe here the main endpoints applied in standard human in vitro models as well as new advanced 3D models that are closer to the in vivo situation. We performed a literature review of in vitro studies published from 2000–2020 (August) dedicated to the genotoxicity of nanomaterials (NMs) in new models. Methods suitable for detection of genotoxicity of NMs will be presented with a focus on advances in miniaturization, organ-on-a-chip and high throughput methods.publishedVersio
Kartlegging av avdampning av kjemikalier fra håndholdte leketøy for barn over 3 år
Get PDFNILU has, on behalf of the Norwegian Environment Agency, performed a screening study to identify volatile organic chemicals (VOCs) emitted from handheld toys for children. The goal was to identify individual VOCs emitted from toys at room temperature and to evaluate what impact the toys may have on the composition and concentrations of VOCs in indoor air. 12-30 individual VOCs were identified in each toy and 65-143 individual VOCs were detected with a concentration higher than 1 µg/m3. VOCs emitted at high concentrations and/or with hazardous properties were cyclohexanone, aromatic VOCs (xylenes, toluene, ethylbenzene), cyclic siloxanes and 2,2,4-Trimethyl-1,3-pentanediol diisobutyrate (TXIB). A regulated hydrochlorofluorocarbon (HCFC-141 b) was also detected from 5 toys. The toys with high concentrations of cyclohexanone and cyclic siloxanes affected the composition and concentrations of VOCs in indoor air.NILU har på oppdrag av Miljødirektoratet utført en kartleggingsstudie av avdampning av flyktige organiske forbindelser (VOC) fra håndholdte leketøy for barn. Formålet med studien var å identifisere enkel-VOCer som dampes av fra leker i romtemperatur og å vurdere påvirkning på sammensetning og nivåer av VOCer i inneluft. 12-30 enkel-VOCer ble identifisert fra hver leke og 65-143 enkel-VOCer med konsentrasjoner høyere enn 1 μg/m3 ble detektert. VOCer som ble målt i høye konsentrsjoner og/eller med helse- og miljøfarlige egenskaper var sykloheksanon, aromatiske VOCer (xylener, toluen, etylbenzen), sykli ske siloks aner and 2,2,4-Trimethyl-1,3-pentanediol diisobutyrate (TXIB). I tilegg ble en regulert hydroklorfluorkarbon (HKFK- 141 b) detektert fra fem leker. Lekene med høyest konsentrasjoner av sykloheksanon og sykliske siloksaner påvirket sammensetningen og konsentrasjonene av VOCer i inneluft.publishedVersio
A review and framework for the evaluation of pixel-level uncertainty estimates in satellite aerosol remote sensing
Get PDFRecent years have seen the increasing inclusion of per-retrieval prognostic (predictive) uncertainty estimates within satellite aerosol optical depth (AOD) data sets, providing users with quantitative tools to assist in optimal use of these data. Prognostic estimates contrast with diagnostic (i.e. relative to some external truth) ones, which are typically obtained using sensitivity and/or validation analyses. Up to now, however, the quality of these uncertainty estimates has not been routinely assessed. This study presents a review of existing prognostic and diagnostic approaches for quantifying uncertainty in satellite AOD retrievals, and presents a general framework to evaluate them, based on the expected statistical properties of ensembles of estimated uncertainties and actual retrieval errors. It is hoped that this framework will be adopted as a complement to existing AOD validation exercises; it is not restricted to AOD and can in principle be applied to other quantities for which a reference validation data set is available. This framework is then applied to assess the uncertainties provided by several satellite data sets (seven over land, five over water), which draw on methods from the empirical to sensitivity analyses to formal error propagation, at 12 Aerosol Robotic Network (AERONET) sites. The AERONET sites are divided into those where it is expected that the techniques will perform well, and those for which some complexity about the site may provide a more severe test. Overall all techniques show some skill in that larger estimated uncertainties are generally associated with larger observed errors, although they are sometimes poorly calibrated (i.e. too small/large in magnitude). No technique uniformly performs best. For powerful formal uncertainty propagation approaches such as Optimal Estimation the results illustrate some of the difficulties in appropriate population of the covariance matrices required by the technique. When the data sets are confronted by a situation strongly counter to the retrieval forward model (e.g. potential mixed land/water surfaces, or aerosol optical properties outside of the family of assumptions), some algorithms fail to provide a retrieval, while others do but with a quantitatively unreliable uncertainty estimate. The discussion suggests paths forward for refinement of these techniques.publishedVersio
Exposure to PFAS is associated with telomere length dynamics and demographic responses of an arctic top predator
Get PDFEnvironmental factors that can influence telomeres are diverse, but the association between telomeres and exposure to environmental contaminants is yet to be elucidated. To date, prior studies have focused on legacy persistent chlorinated pollutants (POPs), while the effects of poly- and perfluoroalkyl substances (PFAS) have been poorly documented. Here, we investigated the associations among PFAS congeners, absolute telomere length (cross-sectional approach), and telomere dynamics (rate of telomere length change over time, longitudinal approach) in one of the most contaminated arctic top predators, the glaucous gull Larus hyperboreus from Svalbard. We further estimated the effect of PFAS on apparent survival rates and re-sighting probabilities using a 10-year capture/recapture dataset (2010–2019). We found that birds exposed to higher concentrations of perfluorononadecanoate (PFNA) (median of 1565 pg/mL of ww in males and 1370 pg/mL of ww in females) and perfluorotetradecanoate (PFTeDA) (median of 370 pg/mL of ww in males and 210 pg/mL of ww in females) showed the slowest rate of telomere shortening. We also found that high blood concentrations of perfluorooctanoate (PFOA) (median of 120 pg/mL of ww in males and 150 pg/mL of ww in females) and perfluorohexanesulfonate (PFHxS) (median of 495 pg/mL of ww in males and 395 pg/mL of ww in females) were positively associated with higher re-sighting probabilities and apparent survival in males but not in females. Our work is the first to report an association between single PFAS compounds and telomeres, and the first to link PFAS exposure with survival probabilities, suggesting that the effect of PFAS exposure might be more tied to the type of compound rather than the total concentration of PFAS.acceptedVersio