1,721,172 research outputs found
Laser ablation parameters influencing gold nanoparticle synthesis in water
The synthesis of gold nanoparticles using pulsed laser ablation in water has special interest in many scientific fields. The nanoparticle production in solution employing an Nd:YAG laser depends mainly on the laser parameters (i.e. by the wavelength, the pulse energy and duration), on the irradiation conditions (target depth in water, focal spot, repetition rate, irradiation time), and on the medium where the ablation occurs (water, solution concentration, presence of surfactants). Optimal conditions can be found in order to control the particle size, the size distribution, and the coalescence effect. A study of these characteristic factors is presented here and discussed
Aluminum ion plasma monitored by SiC detectors from low to high laser intensity and from ns up to fs pulse duration
Thick and thin films of Al targets were irradiated in vacuum with different IR lasers at intensities between 1010 W/cm 2 and 1019 W/cm2, with pulse duration ranging between 3 ns and 45 fs. The laser-generated plasma was monitored in forward and backward directions, from thin and thick targets, by using SiC detectors, ion collectors, ion energy analyzer, optical spectrometer, Thomson parabola spectrometer and X-ray streak camera. Ion emission shows a maximum ion acceleration proportional to the laser intensity, which reaches about 1 MeV per charge state at 1016 W/cm2. Using fs laser, Al ion acceleration occurs at energies up to about 26 MeV and protons are accelerated at energies up to about 2.0 MeV. In the used experimental conditions, the maximum ion acceleration can be controlled by the laser parameters, irradiation conditions, and target geometry, such as the pulse energy, the focal position and the target thickness. Although different lasers and irradiation conditions were employed, the produced ion charges per solid angle of detection remain comparable, as it will be discussed
Laser ablation of boron nitride in vacuum and in water
The laser ablation of boron-nitride (BN) ceramic was employed for the preparation of thin films in high vacuum and nanoparticles and nanocrystals generated in water. The obtained plasma was investigated using ion detectors to determine the ion velocity, the energy per charge state and the plasma temperature and describing the acceleration mechanism. The kinetics of laser ablation in water and the comparison of different ablation rates in the vacuum and in water, and the possible applications of the BN thin film and nanoparticles are presented and discussed
Pulsed laser cleaning (PLC) applied to samples in cultural heritage field
The pulsed laser cleaning (PLC) technique employing different laser wavelengths, with a ns pulse duration, is presented. Such a technique can be applied to the preservation of cultural heritage artworks on different materials, like metals, ceramics and glasses to clean the surfaces of debris accumulated over the years, to remove the oxidation layers, the dust, the organic materials and other unwanted layers, restoring their original composition and shape. PLC should be preceded by surface analyses to control the state of the surface before and during the cleaning process, which has to be carefully controlled, in order to stop the cleaning before to damage the underlying original surface. PLC examples, applied to metals, terracotta and glazy ceramics, are presented and discussed using IR, visible and UV pulsed laser irradiations at low intensity
Protons and carbon ions acceleration in the target-normal-sheath-acceleration regime using low-contrast fs laser and metal-graphene targets
fs pulsed lasers at an intensity of the order of 1018 W/cm2, with a contrast of 10−5, were employed to irradiate thin foils to study the target-normal-sheath-acceleration (TNSA) regime. The forward ion acceleration was investigated using 1/11 μm thickness foils composed of a metallic sheet on which a thin reduced graphene oxide film with 10 nm thickness was deposited by single or both faces. The forward-accelerated ions were detected using SiC semiconductors connected in time-of-flight configuration. The use of intense and long pre-pulse generating the low contrast does not permit to accelerate protons above 1 MeV because it produces a pre-plasma destroying the foil, and the successive main laser pulse interacts with the expanding plasma and not with the overdense solid surface. Experimental results demonstrated that the maximum proton energies of about 700 keV and of 4.2 MeV carbon ions and higher were obtained under the condition of the optimal acceleration procedure. The measurements of ion energy and charge states confirm that the acceleration per charge state is measurable from the proton energy, confirming the Coulomb–Boltzmann-shifted theoretical model. However, heavy ions cannot be accelerated due to their mass and low velocity, which does not permit them to be subjected to the fast and high developed electric field driving the light-ion acceleration. The ion acceleration can be optimized based on the laser focal positioning and on the foil thickness, composition, and structure, as it will be presented and discussed
Six MeV proton acceleration from plasma generated by high-intensity laser using advanced thin polyethylene targets
Proton acceleration can be induced by non-equilibrium plasma developed by high-intensity laser pulses, at 1016 W/cm2, irradiating different types of thin polyethylene targets. The process of proton acceleration and directive yield emission was investigated, optimizing the laser parameters, the irradiation conditions, and the target properties. The use of 600 J pulse energy, a laser focalization inducing self-focusing effects and advanced targets with embedded nanoparticles and optimal thicknesses, has permitted to accelerate forward protons up to the energies of about 6 MeV and amount of the order of 1015 H+/pulse. High proton energy is obtained using thin foils enriched with gold nanoparticles, whereas high proton yield is obtained using targets with a thickness of about 10 μm. The plasma diagnostics using SiC semiconductor detectors in time-of-flight configuration was fundamental to monitor the optimal conditions to improve the plasma processes concerning the ion acceleration and the X-ray and relativistic electron emission
Tantalum ion acceleration in laser-generated plasma and dependence on the pulse duration
The laser irradiation of tantalum targets is presented for different pulsed laser intensities ranging from 1010 up to about 1018 W/cm2 and pulse durations from 9 ns up to 40 fs. The results show that the produced non-equilibrium plasma accelerates Ta ions in the backward direction from values of the order of keV up to values of about 5 MeV. In thin foils, the forward plasma, developed behind the target along the direction of incoming laser, at intensities of about 1016 W/cm2 and 300 ps pulse duration, accelerates Ta ions at energies of the order of 4.6 MeV and produces charge states up to about 40+. For fs lasers at intensities of the order of 1018 W/cm2, only proton acceleration occurs up to 2.1 MeV while no Ta ions are accelerated, due to the reduced duration of the electric field and to the too high inertial mass of the Ta ions
Laser-generated Cu plasma in vacuum and in nitrogen gas
A pulsed ns IR laser at about 1010 W/cm2 intensity is employed to irradiate a Cu target placed in a vacuum and in nitrogen gas. The produced plasma is characterized in terms of emitted ions and photons as a function of the nitrogen pressure in the chamber. The mechanisms of ion gas interactions are investigated in terms of Cu ion energy loss and X-ray attenuation using an ion collector and a SiC detector. A fast CCD camera in the visible region has produced the collision images of the ions with the nitrogen molecules. A plasma temperature of about 44 eV, an emission of soft X-rays up to about 100 eV, an ablation yield of about 2.4 × 1015 atoms/pulse, a maximum Cu ion acceleration of 1.4 keV and a maximum ionization up to Cu9+ were measured in high vacuum
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