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    Enhanced soft dielectric composite generators: the role of ceramic fillers

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    A notable issue in the field of dielectric elastomers is the characterization of composite materials with improved electromechanical coupling destined for mechanical-to-electrostatic energy converters. To this aim, random composites, where ceramic fillers with high dielectric constant are dispersed in a silicone matrix, represent an interesting option. Currently, the most promising reinforcing materials to be immersed in a silicone matrix, already tested for soft dielectric actuators, are lead magnesium niobate–lead titanate (PMN–PT) and lead zirconate-titanate (PZT). To estimate the performance improvement entailed by the composite device with respect to the homogeneous matrix, a typical four-phase cycle is considered in the model, where nominal load and electric charge are alternately held constant. Different materials are being studied: a composite consisting of a matrix in poly-dimethyl-siloxane (PDMS) reinforced with PMN–PT, assuming a filler concentration of 10% in volume and a PDMS–PZT composite with a 1% volume fraction of the ceramic component. In comparison with pure PDMS, the PDMS–10%PMN–PT allows an increase of more than 60% in the harvested energy per unit volume, while the PDMS–1%PZT composite, entailing a minor improvement, here in the range 23.5–37.4%, exhibits a better performance in terms of generated energy per unit weight. These results provide a guide for the choice and design of materials suitable for the realization of enhanced energy harvesters

    The role of electrostriction on the stability of dielectric elastomer actuators

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    AbstractIn the field of soft dielectric elastomers, the notion ‘electrostriction’ indicates the dependency of the permittivity on strain. The present paper is aimed at investigating the effects of electrostriction onto the stability behaviour of homogeneous electrically activated dielectric elastomer actuators. In particular, three objectives are pursued and achieved: (i) the description of the phenomenon within the general nonlinear theory of electroelasticity; (ii) the application of the recently proposed theory of bifurcation for electroelastic bodies in order to determine its role on the onset of electromechanical and diffuse-mode instabilities in prestressed or prestretched dielectric layers; (iii) the analysis of band-localization instability in homogeneous dielectric elastomers. Results for a typical soft acrylic elastomer show that electrostriction is responsible for an enhancement towards diffuse-mode instability, while it represents a crucial property – necessarily to be taken into account – in order to provide a solution to the problem of electromechanical band-localization, that can be interpreted as a possible reason of electric breakdown. A comparison between the buckling stresses of a mechanical compressed slab and the electrically activated counterpart concludes the paper

    Performance of soft dielectric laminated composites

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    This paper contains a thorough investigation of the performance of electrically activated layered soft dielectric composite actuators under plane deformation. Noting that the activation can be induced by controlling either the voltage or the surface charge, the overall behaviour of the system is obtained via homogenization at large strains, taking either the macroscopic electric field or the macroscopic electric displacement field as independent electrical variables. The performance of a two-phase composite actuator compared to that of the homogeneous case is highlighted for few boundary-value problems and for different values of stiffness and permittivity ratios between constituents being significant for applications, where the soft matrix is reinforced by a relatively small volume fraction of a stiff and high-permittivity phase. For charge-controlled devices, it is shown that some composite layouts admit, on one hand, the occurrence of pull-in/snap-through instabilities that can be exploited to design release-actuated systems, and on the other hand, the possibility of thickening at increasing surface charge density
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